While organic chemists are good at synthesizing a variety of small molecules, we fall short of replicating the synthetic precision and fidelity demonstrated by natural enzymes. Nature is truly the best synthetic chemist out there and we draw upon this inspiration to design new catalysts. I will discuss how our team has designed and investigated squishy (polymer-based) homogeneous catalysts that embrace some key design elements found in natural systems to accelerate photoredox reactions and achieve precise bond formation.